I think the 59's would do it. I guarantee you that if Gary Moore was around to pick up a Les Paul with 59's in it and play it for you that it would sound exactly like Gary Moore.
On the other hand, if Eric Clapton were to pick up a Les Paul with 59's in it, plug it in and start playing, it'd sound just like ERIC CLAPTON.
Oh...if Eddie Van Halen picked up that same Les Paul with 59's and started playing, it'd then sound exactly like Eddie.
If I picked it up and started playing it, it wouldn't sound like any of those guys. It'd sound like me.
That said, I'd rather have alnico 2 humbuckers in that Les Paul. Nickel covered Pearly Gates would be just fine.