If you would like to listen to him, I suggest starting with his first two solo albums. The first one is called Neil Young, and the second (the first one with Crazy Horse) is called Everybody Knows This is Nowhere. The first features what I consider to be his best songwriting, and the second is Crazy Horse at their best (semi-retarded, but great, dinosaur jam rock).
Here's one of the songs from the album that your arrangement reminded me of: